At present, there is one train from Barcelona direct to Marseille, leaving at 18.26 and arriving 22.58. There are also some trains with a change in Montpellier. To get to Aix or Avignon, you would have to take an onward train and there are none that would connect with the direct train.
For the best prices, book soon after tickets go on sale, 3 months before travel, with www.capitainetrain.com
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