The Marunouchi Building is right opposite Tokyo Station Marunouchi exit. It gives you the best views of the station at night, with imperial palace gardens opposite.
Casual restaurants are located on floors 5&6, higher end restaurants can be found on the higher floors. We often went for food on the 6th floor at Aoyuzu Tora (see AoyuzuTora review), there is also a really refreshing "western diner" restaurant on either the 5th of 6th, I think it was the 5th. I can't remember the name, but they served an awesome portion of fish & chips and also fresh dough pizza.
There are lots clothes boutiques and beauty treatments. They use OPI nail varnish at the nail bar (but don't have a nail drying machine!! Eating dinner with wet nails and chopsticks was not fun!), there is a massage and hair salon also.
Well worth a stop off after a day of sight seeing.
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