Once you arrive in Sucre you should take some time and visit the Casa de Turismo. Marco the multilingual and established owner and his employee will give you the best tips you can get on Sucre and Bolivia. It seems there's almost nothing Marco doesn't know about this awesome country, be it tours, customs, habits and culture, sights, accommodation, restaurants, bars, language courses, whatsoever; he will get you the right thing.
They will also help you pick the right tour operator which can be really important in Bolivia (safety, price, knowledge, etc). We did the Uyuni-Tour with Red Planet Expeditions on the centre's recommendation and couldn't be more happy with this choice, it was just amazing.
The shop has some really cool souvenirs too and is well located. Please note: the address has changed lately. They aren't in the Calle Bustillos anymore as suggested by tripadvisor but you will find the centre at Calle Audiencia No. 81, which is a 2-minute-stroll uphill from the southern tip of the main square (Plaza 25 de Mayo). Honest, accurate and independent information in Spanish, English, German and French.
Muchas gracias, Marco!
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